Optical and Defect Properties in Nearly Stochiometry ZnO Film Coated on Si (111) by Ultrasonic Spray Pyrolysis Method

Authors

  • Bambang Soegijono Departement of Physics, Universitas Indonesia, Indonesia
  • Hamdan AKbar Notonegoro Department of Mechanical Engineering, Universitas Sultan Ageng Tirtayasa, Indonesia
  • Iwan Sugihartono Departement of Chemistry, Universitas Indonesia, Indonesia
  • Emil Budianto Departement of Chemistry, Universitas Indonesia Depok, Indonesia
  • Muhamad Riza Iskandar 5Central Facility for Electron Microscope, RWTH Aachen University, Germany

DOI:

https://doi.org/10.24203/ajas.v8i4.6291

Keywords:

Keywords— ZnO film, Ultrasonic Spray Pyrolysis , Defect, optical

Abstract

ZnO is one of ceramic semiconductor material, which has interesting properties due its wide bandgap energy (3.4 eV), and it may be used in many optoelectronic devices. Optical and Defects properties of ZnO  could affect the properties of the devices. ZnO films have been deposited on Si (111) substrate by ultrasonic spray pyrolysis (U.S.P.) method at temperatures 400oC, 450oC, and 500oC. The samples consist of two part, annealed and non-annealed heat treatment. The annealed treatment was conducted at temperature 800oC for 2 hours. The XRD pattern revealed that the ZnO film is a polycrystalline. The T.E.M. characterization showed that non stochiometry of the ZnO film present. From the UV-vis pattern, the transition of electrons is affected by the defect present. The ZnO films show a characteristic luminescence properties. It found three defects, there are oxygen vacancies (Vo), oxygen interstitial (Oi), and an electron transition from the level of the ionized oxygen vacancies to the valence band, that is responsible for green band emission.

 

References

M.A Borysiewicz, ZnO as a Functional Materials: A Review, Crystals, 9(10), 505, 2019

X. W. Sun and H. S. Kwok, J. Appl. Phys. 86, 408-411 (1999)

Segawa Y, Ohtomo A, Koinuma M, Tang ZK, Yu P, Wong GKL., Phys Stat Sol (b), 202:669 (1997)

S.T. Tan, B. J. Chen, X. W. Sun, W. J. Fan, H. S. Kwok, X. H. Zhang, and S. J. Chua, J. App. Phys. 98, 013505 (2005)

K.K. Kim, J.H. Song, H.J. Jung, W.K. Choi, S.J. Park, J.H., Song, J. Appl. Phys. 87, 3573(2000).

X. W. Sun and H. S. Kwok, J. Appl. Phys. 86, 408 (1999)

N. Izyumskaya, V. Avrutin, U. Ozgur, Y.I. Alivov, and H. Morkoc, Phys. stat. sol. (b) 244, p. 1439-1450 (2007)

J.L. Zhao, X.W. Sun, S.T. Tan, G.Q. Lo, D.L. Kwong, Z.H. Cen, Appl. Phys. Lett. 91, 263501, (2007).

S. Iwan, S. Bambang, J. L. Zhao, S. T. Tan, X. W. Sun, G.Q. Lo, H. M. Fan, L. Sun, S. Zhang, Physica B, 407, 2721-2724 (2012)

P.T. Hsieh, Y.C. Chen, K.S. Kao, M.S. Lee, C.C. Cheng, J. European Ceramic Society, 27, 3815-3818 (2007)

A. van Dijken, E.A. Meulenkamp, D. Vanmaekelbergh, A. Meijerink, J. Luminescence 20, 123-128 (2000)

Q.P. Wang, D.H. Z.Y. Z.Y. Xue, and X.T. Hao, Appl. Surface Science 201, p.123-128 (2002)

D. C. Look, B. Claflin, Ya. I. Alivov, and S. J. Park, Phys. Stat. sol. (a) 201, 2203–2212 (2004).

X.M. Fan, J.S. Lian, Z.X. Guo, and H.J. Lu, Appl. Surface Science 239, p.176-181 (2005)

B. Lin, Z. Fu, Y. Jia, Appl. Phys. Lett. 79, 943 (2001)

M. Liu, A.H. Kitai, P. Mascher, J. Luminescence 54, 35 (1992)

Y.M. Sun, Ph.D. Thesis, University of Science, and Technologyof China (2000).

Iwan Sugihartono, Bambang Soegijono, M. Hikam, E. Handoko, Fan H.M, S.T. Tan, X.W. Sun, 2013 International Confrence on QiR, p. 232-234 (2013)

D.H. Zhang, Z.Y. Xue, Q.P. Wang, J. Ma, Proc. SPIE 4918, 425 (2002)

K. Vanheusden, W.L. Warren, C.H. Seage, D.R. Tallent, J.A.Voigtang, B.E. Gnade, J.Appl. Phys. 79, 7983 (1996).

Downloads

Published

2020-08-28

How to Cite

Soegijono, B., Notonegoro, H. A., Sugihartono, I., Budianto, E., & Iskandar, M. R. (2020). Optical and Defect Properties in Nearly Stochiometry ZnO Film Coated on Si (111) by Ultrasonic Spray Pyrolysis Method. Asian Journal of Applied Sciences, 8(4). https://doi.org/10.24203/ajas.v8i4.6291

Issue

Vol. 8 No. 4 (2020): August 2020

Section

Articles

License

Copyright (c) 2020 Bambang Soegijono, Hamdan AKbar Notonegoro, Iwan Sugihartono, Emil Budianto, Muhamad Riza Iskandar

Creative Commons License

This work is licensed under a Creative Commons Attribution-NonCommercial 4.0 International License.

  • Papers must be submitted on the understanding that they have not been published elsewhere (except in the form of an abstract or as part of a published lecture, review, or thesis) and are not currently under consideration by another journal published by any other publisher.
  • It is also the authors responsibility to ensure that the articles emanating from a particular source are submitted with the necessary approval.
  • The authors warrant that the paper is original and that he/she is the author of the paper, except for material that is clearly identified as to its original source, with permission notices from the copyright owners where required.
  • The authors ensure that all the references carefully and they are accurate in the text as well as in the list of references (and vice versa).
  • Authors retain copyright and grant the journal right of first publication with the work simultaneously licensed under a Attribution-NonCommercial 4.0 International that allows others to share the work with an acknowledgement of the work's authorship and initial publication in this journal.
  • Authors are able to enter into separate, additional contractual arrangements for the non-exclusive distribution of the journal's published version of the work (e.g., post it to an institutional repository or publish it in a book), with an acknowledgement of its initial publication in this journal.
  • Authors are permitted and encouraged to post their work online (e.g., in institutional repositories or on their website) prior to and during the submission process, as it can lead to productive exchanges, as well as earlier and greater citation of published work (See The Effect of Open Access).
  • The journal/publisher is not responsible for subsequent uses of the work. It is the author's responsibility to bring an infringement action if so desired by the author.

Most read articles by the same author(s)